Radiochemistry

Research output

Research output per year 2014 2019 2020 2021 2022 2023 2024

• 49 Article
• 21 In-proceedings paper
• 12 Doctoral thesis
• 8 ER - External report
• 16 More
  • 7 Master's thesis
  • 5 Literature review
  • 2 Professional Bachelor's thesis
  • 1 Chapter
  • 1 Special issue

Research output per year

Research output per year

Search results

• 2024

  Development and preclinical evaluation of 161Tb radiopharmaceuticals for cancer treatment

  Cassells, I. & Ooms, M. (Peer reviewer), 24 Jun 2024, KUL - Katholieke Universiteit Leuven. 173 p.

  Research output

• Electrolytic reduction in LiCl-Li2O of titania microspheres synthesized via vibrational droplet coagulation: Effect of feed morphology

  Hsu, H.-H., Breugelmans, T., Cardinaels, T. & Geboes, B., Jun 2024, In: Journal of Industrial and Engineering Chemistry. 3 p.

  Research output › peer-review

• Improving americium/curium separation factors in the AmSel process through symmetry lowering of the diglycolamide extractant

  Kolesar, F., Van Hecke, K., Verguts, K., Marie, C., Berthon, L., Binnemans, K. & Cardinaels, T., Nov 2024, In: ACS Omega. 14 p., 4c06426.

  Research output › peer-review

  Open Access

• Influence of the gamma source on the radiolytic stability of N,N,N′,N′-tetra-n-octyl-diglycolamide (TODGA)

  Verguts, K., Van Hecke, K., Jordens, J., Voorspoels, S. & Cardinaels, T., Nov 2024, In: Radiochimica Acta. 5 p.

  Research output › peer-review

  Open Access

• Investigating D2EHBA as extractant for uranium/plutonium co-extraction with annular centrifugal contactors

  Cosemans, S., Maertens, D. (Peer reviewer) & Cardinaels, T. (Peer reviewer), 7 Jun 2024, KUL - Katholieke Universiteit Leuven. 91 p.

  Research output

• Kinetics of electrochemical Eu³⁺ to Eu²⁺ reduction in aqueous media

  Arman, M. Ö., Geboes, B., Van Hecke, K., Binnemans, K. & Cardinaels, T., 20 Apr 2024, In: Electrochimica Acta. 484, 10 p., 144055.

  Research output › peer-review

• Separation of terbium as a first step towards high purity terbium-161 for medical applications

  Arman, M., Mullaliu, A., Geboes, B., Van Hecke, K., Das, G., Aquilanti, G., Binnemans, K. & Cardinaels, T., 20 Jun 2024, In: RSC Advances. 14, 28, p. 19926-19934 9 p.

  Research output › peer-review

  Open Access

• Validation of concept continuous counter-current separation of Platinum Group Metals and Am(III) from a simulated high active raffinate solution: Centrifugal contactor development and solvent extraction studies

  Zsabka, P., 20 Feb 2024, SCK CEN. 19 p. (SCK CEN Reports; no. ER-1391)

  Research output › peer-review

  Open Access

  File
  16 Downloads (Pure)
• 2023

  ²³⁸Pu production:a State-of-the-Art review of NpO2 target fabrication technologies and processing of irradiated targetsA State-of-the-Art review of NpO₂target fabrication technologies and processing of irradiated targets

  Acevedo Muñoz, B., Van Hecke, K., Cardinaels, T. & Verwerft, M., 1 Dec 2023, In: Radiochimica Acta. 111, 12, p. 857-885 29 p.

  Research output › peer-review

• 3p-C-NETA-TATE: a theranostic somatostatin analogue targeting neuroendocrine tumors

  Ahenkorah, S., Murce, E., Cawthorne, C., Seimbille, Y., Cardinaels, T., Deroose, C., Bormans, G., Ooms, M. & Cleeren, F., 15 Jun 2023, Abstracts from the 20th European symposium on radiopharmacy and radiopharmaceuticals. 1 ed. Springer, Vol. 8. p. 6-6 1 p. OP13. (EJNMMI Radiopharmacy and Chemistry ; vol. 8, no. Supplement 1).

  Research output › peer-review

  Open Access

• Adsorption of radon on silver exchanged zeolites at ambient temperatures

  Heinitz, S., Mermans, J., Maertens, D., Skliarova, H., Aerts, A., Cardinaels, T., Gueibe, C., Rutten, J., Ireland, N., Kuznicki, D. & Kuznicki, S., Dec 2023, In: Scientific Reports. 13, 1, 11 p., 6811.

  Research output › peer-review

  Open Access

• Beyond U/Pu separation: separation of americium from the highly active PUREX raffinate

  Zsabka, P., Wilden, A., Van Hecke, K., Modolo, G., Verwerft, M. & Cardinaels, T., 1 Aug 2023, In: Journal of Nuclear Materials. 581, 1 p., 154445.

  Research output › peer-review

  Open Access

• Carbon materials tailored for 225Ac/213Bi separation and their use in radionuclide generators

  Zhu, H., Cardinaels, T. (Peer reviewer) & Heinitz, S. (Peer reviewer), Jul 2023, KUL - Katholieke Universiteit Leuven. 298 p.

  Research output

  Open Access

  File
  11 Downloads (Pure)

• De invloed van fasemodificatoren in het AmSel proces

  Put, W., Van Hecke, K. (Peer reviewer), Verguts, K. (Peer reviewer) & Kolesar, F. (Peer reviewer), 23 Jun 2023, Thomas More. 51 p.

  Research output

  Open Access

  File
  16 Downloads (Pure)

• Design of a modular annular centrifugal contactor for lab-scale counter-current multistage solvent extraction

  Maertens, D., Binnemans, K. & Cardinaels, T., 1 Aug 2023, In: Solvent extraction and ion exchange. 41, 6, p. 741-766 26 p.

  Research output › peer-review

  Open Access

• Direct comparison of [18F]AlF-NOTA-JR11 and [18F]AlF-NOTA-octreotide for PET imaging of neuroendocrine tumors: Antagonist versus agonist

  Ahenkorah, S., Cawthorne, C., Murce, E., Deroose, C., Cardinaels, T., Seimbille, Y., Bomans, G., Ooms, M. & Cleeren, F., 1 Mar 2023, In: Nuclear Medicine and Biology. 118-119, 10 p., 108338.

  Research output › peer-review

  Open Access

• Feasibility evaluation on European capabilities for 238Pu based radioisotope power systems

  Acevedo Muñoz, B., Romojaro, P., Van den Eynde, G., Van Hecke, K., Cardinaels, T. & Verwerft, M., 6 Nov 2023, 2023 13th European Space Power Conference, ESPC 2023. 2023 ed. Elche, Spain: Institute of Electrical and Electronics Engineers Inc., 13 p. (2023 13th European Space Power Conference, ESPC 2023).

  Research output › peer-review

• First-principles study of the radiolytic degradation of diglycolamides

  Verlinden, B., Van Hecke, K., Wilden, A., Modolo, G., Binnemans, K., Cardinaels, T. & Kowalski, P. M., 1 Oct 2023, In: Radiochimica Acta. 111, 10, p. 741-750 10 p.

  Research output › peer-review

• Gamma radiation effects on AG MP-50 cation exchange resin and sulfonated activated carbon for bismuth-213 separation

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Derveaux, E., Adriaensens, P., Binnemans, K., Mullens, S. & Cardinaels, T., 24 Oct 2023, In: RSC Advances. 13, 44, p. 30990-31001 12 p.

  Research output › peer-review

  Open Access

• P-232 - Nanosized crystalline vehicle for targeted radionuclide therapy

  Lemaître, T., Opsomer, T., Ooms, M., Burgoyne, A., Van de Voorde, M., Cardinaels, T. & Parac-Vogt, T. N., 1 Dec 2023, Nuclear Medicine and Biology: Abstracts of the International Symposium on Radiopharmaceutical Sciences iSRS 2023. Supplement ed. Elsevier, Vol. 126–127. p. S226 1 p. 108696. (Nuclear Medicine and Biology; vol. 126-127).

  Research output › peer-review

  Open Access

• Selective separation of Bi³⁺ from La³⁺/Ac³⁺ by sorption on sulfonated carbon materials for use in an inverse ²²⁵Ac/²¹³Bi radionuclide generator: Batch and column tests

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Binnemans, K., Mullens, S. & Cardinaels, T., 15 Jul 2023, In: Chemical Engineering Journal. 468, 15 p., 143416.

  Research output › peer-review

  Open Access

• Separation of americium from highly active raffinates by an innovative variant of the AmSel process based on the ionic liquid Aliquat-336 nitrate

  Kolesar, F., Van Hecke, K., Zsabka, P., Binnemans, K. & Cardinaels, T., 12 Dec 2023, In: RSC Advances. 13, 51, p. 36322-36336 15 p.

  Research output › peer-review

  Open Access

• Solvent Optimization Studies for a New EURO- GANEX Process with 2,2’-Oxybis(N,N-di-ndecylpropanamide) (mTDDGA) and Its Radiolysis Products

  Verlinden, B., Wilden, A., Van Hecke, K., Egberink, R. J. M., Huskens, J., Verboom, W., Hupert, M., Weßling, P., Geist, A., Panak, P. J., Hermans, R., Verwerft, M., Modolo, G., Binnemans, K. & Cardinaels, T., Jan 2023, In: Solvent extraction and ion exchange. 41, 1, p. 59-87 29 p.

  Research output › peer-review

  Open Access

• Sorption and desorption performance of La3+/Bi3+ by surface-modified activated carbon for potential application in medical 225Ac/213Bi generators

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Binnemans, K., Mullens, S. & Cardinaels, T., 15 May 2023, In: Chemical Engineering Journal. 464, 14 p., 142456.

  Research output › peer-review

  Open Access

• Tuning oxidation states of terbium and europium towards high purity terbium-161 and samarium-153 for medical applications

  Arman, M., Cardinaels, T. (Peer reviewer), Geboes, B. (Peer reviewer) & Van Hecke, K. (Peer reviewer), 28 Sep 2023, KUL - Katholieke Universiteit Leuven. 214 p.

  Research output

  Open Access

  File
  178 Downloads (Pure)
• 2022

  3p-C-NETA: A versatile and effective chelator for development of Al¹⁸F-labeled and therapeutic radiopharmaceuticals

  Ahenkorah, S., Murce, E., Cawthorne, C., Ketchemen, J. P., Deroose, C. M., Cardinaels, T., Seimbille, Y., Fonge, H., Gsell, W., Bormans, G., Ooms, M. & Cleeren, F., 2022, In: Theranostics. 12, 13, p. 5971-5985 15 p.

  Research output › peer-review

  Open Access
  7 Scopus citations

• 3p-C-NETA-TATE: a versatile somatostatin analogue for Al18F-labeled and therapeutic SSTR2 targeting radiopharmaceuticals

  Ahenkorah, S., Murce, E., Ketchemen, J., Cawthorne, C., Seimbille, Y., Cardinaels, T., Bormans, G., Fonge, H., Ooms, M. & Cleeren, F., May 2022, Abstracts of the International Symposium on Radiopharmaceutical Sciences iSRS 2022. Supplement ed. Elsevier, Vol. 108-109. p. S10-S11 2 p. O-11. (Nuclear Medicine and Biology).

  Research output › peer-review

  Open Access

• Bifunctional chelators for radiorhenium: past, present and future outlook

  Melis, D., Burgoyne, A., Ooms, M. & Gasser, G., 14 Jan 2022, In: RSC Medicinal Chemistry. 13, 3, p. 217-245 29 p.

  Research output › peer-review

  Open Access

• Development of an in-house 188W/188Re generator for rhenium-188 production and radiolabelling studies

  Melis, D., Opsomer, T., Ponsard, B., Burgoyne, A., Gasser, G., Van de Voorde, M. & Ooms, M., Dec 2022, Nuclear Medicine and Biology: Abstracts of the Fourth International Symposium on Technetium and Other Radiometals in Chemistry and Medicine (TERACHEM 2022). Elsevier, Vol. 114-115/S. p. S38 1 p. P-11. (Nuclear Medicine and Biology; vol. 114-115/S).

  Research output › peer-review

  Open Access

• Development of targeted 161Tb-radiolabeled nanoparticles

  Lemaître, T., Ooms, M., Opsomer, T., Van de Voorde, M., Cardinaels, T. & Parac-Vogt, T. N., 1 Dec 2022, Nuclear Medicine and Biology: Abstracts of the Fourth International Symposium on Technetium and Other Radiometals in Chemistry and Medicine (TERACHEM 2022). Elsevier, Vol. 114-115/S. p. S69 1 p. P-73. (Nuclear Medicine and Biology; vol. 114-115/S).

  Research output › peer-review

  Open Access

• Development of theranostic somatostatin analogues for the treatment of neuroendocrine tumors

  Ahenkorah, S., Ooms, M. (Peer reviewer) & Cardinaels, T. (Peer reviewer), 15 Dec 2022, 178 p.

  Research output

  Open Access

• Effect of ionizing radiation on solvent extraction systems for the separation of minor actinides

  Verlinden, B., Cardinaels, T. (Peer reviewer) & Van Hecke, K. (Peer reviewer), 28 Feb 2022, KUL - Katholieke Universiteit Leuven. 194 p.

  Research output

  Open Access

  File
  21 Downloads (Pure)

• Effect of metal impurities on the radiolabeling efficiency of DOTA with terbium-161 and lutetium-177: a comparative study

  Opsomer, T., Van de Voorde, M., Vermeulen, K., Ramaekers, S., Burgoyne, A. & Ooms, M., 8 Dec 2022, Nuclear Medicine and Biology: Abstracts of the Fourth International Symposium on Technetium and Other Radiometals in Chemistry and Medicine (TERACHEM 2022). 2022 ed. Elsevier, Vol. 114-115/S. p. S57-S58 2 p. P-53. (Nuclear Medicine and Biology; vol. 114-115/S).

  Research output › peer-review

  Open Access

• Electrochemical oxidation of terbium(III) in aqueous media: influence of supporting electrolyte on oxidation potential and stability

  Arman, M., Geboes, B., Van Hecke, K., Binnemans, K. & Cardinaels, T., 11 Jan 2022, In: Journal of Applied Electrochemistry. 52, p. 583-593 11 p.

  Research output › peer-review

  Open Access

• Evaluating the in vivo distribution and stability of a 161Tb-labeled nanobody for potential cancer therapy

  Cassells, I., Van de Voorde, M., Vermeulen, K., Rodriguez Pérez, S., Segers, C., Cawthorne, C., Deroose, C., Cardinaels, T., Bormans, G., Ooms, M. & Cleeren, F., 8 Dec 2022, Nuclear Medicine and Biology: Abstracts of the Fourth International Symposium on Technetium and Other Radiometals in Chemistry and Medicine (TERACHEM 2022). Elsevier, Vol. 114-115/S. p. S50 1 p. P-37. (Nuclear Medicine and Biology; vol. 114-115/S).

  Research output › peer-review

  Open Access

• Evaluation of 3p-C-DEPA as potential 225Ac-chelator

  Ahenkorah, S., Ramdhani, D., Deroose, C., Cardinaels, T., Bormans, G., Cleeren, F. & Ooms, M., 8 Dec 2022, Nuclear Medicine and Biology: Abstracts of the Fourth International Symposium on Technetium and Other Radiometals in Chemistry and Medicine (TERACHEM 2022). Elsevier, Vol. 114-115/S. p. S49 1 p. P-35. (Nuclear Medicine and Biology; vol. 114-115S).

  Research output › peer-review

  Open Access

• Evaluation of the irradiation-averaged fission yield for burnup determination in spent fuel assays

  Govers, K., Adriaensen, L., Dobney, A., Gysemans, M., Cachoir, C. & Verwerft, M., 13 Sep 2022, In: EPJ N - Nuclear Sciences and Technologies. 8, p. 1-15 15 p., 18.

  Research output › peer-review

  Open Access

• Exploring the potential of high-molar activity Samarium-153 for targeted radionuclide therapy with [153Sm]Sm-DOTA-TATE

  Vermeulen, K., Van de Voorde, M., Segers, C., Coolkens, A., Rodriguez Perez, S., Duchemin, C., Crabbé, M., Opsomer, T., Saldarriaga Vargas, C., Reinhard, H., Lambert, L., Bernerd, C., Burgoyne, A., Cocolios, T. E., Stora, T. & Ooms, M., 18 Nov 2022, In: Pharmaceutics. 14, p. 1-15 15 p., 2566.

  Research output › peer-review

  Open Access

• Gamma counting protocols for the accurate quantification of 225Ac and 213Bi without the need for a secular equilibrium between parent and gamma‑emitting daughter

  Castillo, D., De Saint-Hubert, M., Ahenkorah, S., Saldarriaga Vargas, C., Ooms, M., Struelens, L. & Koole, M., 23 Oct 2022, In: EJNMMI Radiopharmacy and Chemistry. 7, 28, 17 p., 28.

  Research output › peer-review

  Open Access

• Gamma radiolytic stability of the novel modified diglycolamide 2,20-oxybis(N,Ndidecylpropanamide) (mTDDGA) for grouped actinide extraction

  Verlinden, B., Van Hecke, K., Wilden, A., Hupert, M., Santiago-Schübel, B., Egberink, R. J. M., Verboom, W., Kowalski, P., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 25 Apr 2022, In: RSC Advances. 12, 20, p. 12416-12426 11 p.

  Research output › peer-review

  Open Access

• Hydrolysis of uranyl-, Nd-, Ce-ions and their mixtures by thermal decomposition of urea

  Schreinemachers, C., Bollen, O., Leinders, G., Tyrpekl, V., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 8 Feb 2022, In: European journal of inorganic chemistry. 2022, 4, 13 p., e202100453.

  Research output › peer-review

  Open Access

• Inorganic Radiolabeled Nanomaterials in Cancer Therapy: A Review

  Lemaître, T., Burgoyne, A., Ooms, M., Parac-Vogt, T. N. & Cardinaels, T., 22 Jun 2022, In: ACS Applied Nano Materials. 5, 7, p. 8560-8709 30 p.

  Research output › peer-review

  Open Access

• Mild condition radiolabelling and in vivo stability of nanobody constructs with terbium-161 and terbium-155

  Cassells, I., Van de Voorde, M., Webster, B., Ivanov, P., Burgoyne, A., Cawthorne, C., Deroose, C., Cardinaels, T., Bormans, G., Cleeren, F. & Ooms, M., 22 May 2022, Nuclear Medicine and Biology. Supplement ed. Elsevier, Vol. 108-109. p. S53-S54 2 p. P-004. (Nuclear Medicine and Biology; vol. 108).

  Research output › peer-review

  Open Access

• O-27 - Using high-specific activity Samarium-153 for the development of [153Sm] Sm DOTA-TATE for targeted radionuclide therapy of neuroendocrine tumors

  Vermeulen, K., Van de Voorde, M., Daems, N., Duchemin, C., Rodriguez Pérez, S., Crabbé, M., Reinhard, H., Ponsard, B., Geenen, L., Nonnekens, J., Lambert, L., Bernerd, C., Burgoyne, A., Cocolios, T. E., Stora, T. & Ooms, M., May 2022, In: Nuclear Medicine and Biology. 108-109, Supplement, p. S20 1 p.

  Research output › peer-review

  Open Access

• Progress in experimental results of the combined Cs/Sr partitioning: ASOF deliverable D 1.2.2

  Verguts, K., 12 Dec 2022, SCK CEN. 8 p. (SCK CEN Reports; no. ER-1212)

  Research output › peer-review

  Open Access

  File
  12 Downloads (Pure)

• Reference composition of the fission product and rest waste stream: ASOF WP3

  Lemmens, K. & Van Hecke, K., 12 Dec 2022, SCK CEN. 19 p. (SCK CEN Reports; no. ER-1190)

  Research output › peer-review

  Open Access

  File
  16 Downloads (Pure)
• 2021

  225Ac labeled anti-HER2 2Rs15d sdAb as a potential therapeutic for targeted alpha therapy – an in vitro and in vivo evaluation

  Rodak, M., Dekempeneer, Y., Wojewodzka, M., Lahoutte, T., Bruchertseifer, F., Morgenstern, A., D'Huyvetter, M. & Pruszynski, M., 21 May 2021, Nuclear Medicine and Biology. Elsevier, Vol. 97-97. p. S33 1 p. SSP-30. (Nuclear Medicine and Biology; vol. 96-97, no. S33).

  Research output › peer-review

  Open Access

• Al18F-3p-C-NETA-TATE: Combining a versatile and highly effective chelator with an established somatostatin analogue

  Ahenkorah, S., Murce, E., Seimbille, Y., Cardinaels, T., Deroose, C., Bormans, G., Ooms, M. & Cleeren, F., 24 Sep 2021, European Journal of Nuclear Medicine and Molecular Imaging: European Association of Nuclear Medicine October 20-23, 2021 Virtual. Springer, Vol. 48. p. S195-S196 1 p. OP-0556. (European Journal of Nuclear Medicine and Molecular Imaging; vol. 48, no. Supplement Issue 1).

  Research output › peer-review

  Open Access

• Bismuth-213 for Targeted Radionuclide Therapy: From Atom to Bedside

  Ahenkorah, S., Cassells, I., Deroose, C., Cardinaels, T., Burgoyne, A., Bormans, G., Ooms, M. & Cleeren, F., 21 Apr 2021, In: Pharmaceutics. 13, 599, p. 1-25 25 p., 599.

  Research output › peer-review

  Open Access

• Dosimetry and methodology of gamma irradiation for degradation studies on solvent extraction systems

  Verlinden, B., Zsabka, P., Van Hecke, K., Verguts, K., Mihailescu, C., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 2021, In: Radiochimica Acta. 109, 1, p. 61-72 12 p.

  Research output › peer-review

  Open Access