Radiochemistry

Research output

Research output per year 2014 2019 2020 2021 2022 2023 2024

• 49 Article
• 21 In-proceedings paper
• 12 Doctoral thesis
• 8 ER - External report
• 16 More
  • 7 Master's thesis
  • 5 Literature review
  • 2 Professional Bachelor's thesis
  • 1 Chapter
  • 1 Special issue

Research output per year

Research output per year

Search results

• 2024

  Electrolytic reduction in LiCl-Li2O of titania microspheres synthesized via vibrational droplet coagulation: Effect of feed morphology

  Hsu, H.-H., Breugelmans, T., Cardinaels, T. & Geboes, B., Jun 2024, In: Journal of Industrial and Engineering Chemistry. 3 p.

  Research output › peer-review

• Improving americium/curium separation factors in the AmSel process through symmetry lowering of the diglycolamide extractant

  Kolesar, F., Van Hecke, K., Verguts, K., Marie, C., Berthon, L., Binnemans, K. & Cardinaels, T., Nov 2024, In: ACS Omega. 14 p., 4c06426.

  Research output › peer-review

  Open Access

• Influence of the gamma source on the radiolytic stability of N,N,N′,N′-tetra-n-octyl-diglycolamide (TODGA)

  Verguts, K., Van Hecke, K., Jordens, J., Voorspoels, S. & Cardinaels, T., Nov 2024, In: Radiochimica Acta. 5 p.

  Research output › peer-review

  Open Access

• Kinetics of electrochemical Eu³⁺ to Eu²⁺ reduction in aqueous media

  Arman, M. Ö., Geboes, B., Van Hecke, K., Binnemans, K. & Cardinaels, T., 20 Apr 2024, In: Electrochimica Acta. 484, 10 p., 144055.

  Research output › peer-review

• Separation of terbium as a first step towards high purity terbium-161 for medical applications

  Arman, M., Mullaliu, A., Geboes, B., Van Hecke, K., Das, G., Aquilanti, G., Binnemans, K. & Cardinaels, T., 20 Jun 2024, In: RSC Advances. 14, 28, p. 19926-19934 9 p.

  Research output › peer-review

  Open Access
• 2023

  Adsorption of radon on silver exchanged zeolites at ambient temperatures

  Heinitz, S., Mermans, J., Maertens, D., Skliarova, H., Aerts, A., Cardinaels, T., Gueibe, C., Rutten, J., Ireland, N., Kuznicki, D. & Kuznicki, S., Dec 2023, In: Scientific Reports. 13, 1, 11 p., 6811.

  Research output › peer-review

  Open Access

• Design of a modular annular centrifugal contactor for lab-scale counter-current multistage solvent extraction

  Maertens, D., Binnemans, K. & Cardinaels, T., 1 Aug 2023, In: Solvent extraction and ion exchange. 41, 6, p. 741-766 26 p.

  Research output › peer-review

  Open Access

• Direct comparison of [18F]AlF-NOTA-JR11 and [18F]AlF-NOTA-octreotide for PET imaging of neuroendocrine tumors: Antagonist versus agonist

  Ahenkorah, S., Cawthorne, C., Murce, E., Deroose, C., Cardinaels, T., Seimbille, Y., Bomans, G., Ooms, M. & Cleeren, F., 1 Mar 2023, In: Nuclear Medicine and Biology. 118-119, 10 p., 108338.

  Research output › peer-review

  Open Access

• First-principles study of the radiolytic degradation of diglycolamides

  Verlinden, B., Van Hecke, K., Wilden, A., Modolo, G., Binnemans, K., Cardinaels, T. & Kowalski, P. M., 1 Oct 2023, In: Radiochimica Acta. 111, 10, p. 741-750 10 p.

  Research output › peer-review

• Gamma radiation effects on AG MP-50 cation exchange resin and sulfonated activated carbon for bismuth-213 separation

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Derveaux, E., Adriaensens, P., Binnemans, K., Mullens, S. & Cardinaels, T., 24 Oct 2023, In: RSC Advances. 13, 44, p. 30990-31001 12 p.

  Research output › peer-review

  Open Access

• Selective separation of Bi³⁺ from La³⁺/Ac³⁺ by sorption on sulfonated carbon materials for use in an inverse ²²⁵Ac/²¹³Bi radionuclide generator: Batch and column tests

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Binnemans, K., Mullens, S. & Cardinaels, T., 15 Jul 2023, In: Chemical Engineering Journal. 468, 15 p., 143416.

  Research output › peer-review

  Open Access

• Separation of americium from highly active raffinates by an innovative variant of the AmSel process based on the ionic liquid Aliquat-336 nitrate

  Kolesar, F., Van Hecke, K., Zsabka, P., Binnemans, K. & Cardinaels, T., 12 Dec 2023, In: RSC Advances. 13, 51, p. 36322-36336 15 p.

  Research output › peer-review

  Open Access

• Solvent Optimization Studies for a New EURO- GANEX Process with 2,2’-Oxybis(N,N-di-ndecylpropanamide) (mTDDGA) and Its Radiolysis Products

  Verlinden, B., Wilden, A., Van Hecke, K., Egberink, R. J. M., Huskens, J., Verboom, W., Hupert, M., Weßling, P., Geist, A., Panak, P. J., Hermans, R., Verwerft, M., Modolo, G., Binnemans, K. & Cardinaels, T., Jan 2023, In: Solvent extraction and ion exchange. 41, 1, p. 59-87 29 p.

  Research output › peer-review

  Open Access

• Sorption and desorption performance of La3+/Bi3+ by surface-modified activated carbon for potential application in medical 225Ac/213Bi generators

  Zhu, H., Heinitz, S., Eyley, S., Thielemans, W., Binnemans, K., Mullens, S. & Cardinaels, T., 15 May 2023, In: Chemical Engineering Journal. 464, 14 p., 142456.

  Research output › peer-review

  Open Access
• 2022

  3p-C-NETA: A versatile and effective chelator for development of Al¹⁸F-labeled and therapeutic radiopharmaceuticals

  Ahenkorah, S., Murce, E., Cawthorne, C., Ketchemen, J. P., Deroose, C. M., Cardinaels, T., Seimbille, Y., Fonge, H., Gsell, W., Bormans, G., Ooms, M. & Cleeren, F., 2022, In: Theranostics. 12, 13, p. 5971-5985 15 p.

  Research output › peer-review

  Open Access
  7 Scopus citations

• Bifunctional chelators for radiorhenium: past, present and future outlook

  Melis, D., Burgoyne, A., Ooms, M. & Gasser, G., 14 Jan 2022, In: RSC Medicinal Chemistry. 13, 3, p. 217-245 29 p.

  Research output › peer-review

  Open Access

• Electrochemical oxidation of terbium(III) in aqueous media: influence of supporting electrolyte on oxidation potential and stability

  Arman, M., Geboes, B., Van Hecke, K., Binnemans, K. & Cardinaels, T., 11 Jan 2022, In: Journal of Applied Electrochemistry. 52, p. 583-593 11 p.

  Research output › peer-review

  Open Access

• Evaluation of the irradiation-averaged fission yield for burnup determination in spent fuel assays

  Govers, K., Adriaensen, L., Dobney, A., Gysemans, M., Cachoir, C. & Verwerft, M., 13 Sep 2022, In: EPJ N - Nuclear Sciences and Technologies. 8, p. 1-15 15 p., 18.

  Research output › peer-review

  Open Access

• Exploring the potential of high-molar activity Samarium-153 for targeted radionuclide therapy with [153Sm]Sm-DOTA-TATE

  Vermeulen, K., Van de Voorde, M., Segers, C., Coolkens, A., Rodriguez Perez, S., Duchemin, C., Crabbé, M., Opsomer, T., Saldarriaga Vargas, C., Reinhard, H., Lambert, L., Bernerd, C., Burgoyne, A., Cocolios, T. E., Stora, T. & Ooms, M., 18 Nov 2022, In: Pharmaceutics. 14, p. 1-15 15 p., 2566.

  Research output › peer-review

  Open Access

• Gamma counting protocols for the accurate quantification of 225Ac and 213Bi without the need for a secular equilibrium between parent and gamma‑emitting daughter

  Castillo, D., De Saint-Hubert, M., Ahenkorah, S., Saldarriaga Vargas, C., Ooms, M., Struelens, L. & Koole, M., 23 Oct 2022, In: EJNMMI Radiopharmacy and Chemistry. 7, 28, 17 p., 28.

  Research output › peer-review

  Open Access

• Gamma radiolytic stability of the novel modified diglycolamide 2,20-oxybis(N,Ndidecylpropanamide) (mTDDGA) for grouped actinide extraction

  Verlinden, B., Van Hecke, K., Wilden, A., Hupert, M., Santiago-Schübel, B., Egberink, R. J. M., Verboom, W., Kowalski, P., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 25 Apr 2022, In: RSC Advances. 12, 20, p. 12416-12426 11 p.

  Research output › peer-review

  Open Access

• Hydrolysis of uranyl-, Nd-, Ce-ions and their mixtures by thermal decomposition of urea

  Schreinemachers, C., Bollen, O., Leinders, G., Tyrpekl, V., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 8 Feb 2022, In: European journal of inorganic chemistry. 2022, 4, 13 p., e202100453.

  Research output › peer-review

  Open Access
• 2021

  Dosimetry and methodology of gamma irradiation for degradation studies on solvent extraction systems

  Verlinden, B., Zsabka, P., Van Hecke, K., Verguts, K., Mihailescu, C., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 2021, In: Radiochimica Acta. 109, 1, p. 61-72 12 p.

  Research output › peer-review

  Open Access

• Production of Sm-153 With Very High Specific Activity for Targeted Radionuclide Therapy

  Van de Voorde, M., Duchemin, C., Reinhard, H., Lambert, L., Chevallay, E., Schneider, T., Van Stenis, M., Cocolios, T. E., Cardinaels, T., Ponsard, B., Ooms, M., Stora, T. & Burgoyne, A., 19 Jul 2021, In: Frontiers in Medicine. 8, p. 1-9 9 p., 675221.

  Research output › peer-review

  Open Access

• Quantification of boron in cells for evaluation of drug agents used in boron neutron capture therapy

  Verlinden, B., Van Hoecke, K., Aerts, A., Daems, N., Dobney, A., Janssens, K. & Cardinaels, T., 14 Jan 2021, In: Journal of Analytical Atomic Spectrometry. 36, 3, p. 598-606 9 p.

  Research output › peer-review

  Open Access

• Radiolabeling of human serum albumin with terbium-161 using mild conditions and evaluation of in vivo Stability

  Cassells, I., Ahenkorah, S., Burgoyne, A., Van de Voorde, M., Deroose, C., Cardinaels, T., Bormans, G., Ooms, M. & Cleeren, F., 18 Aug 2021, In: Frontiers in Medicine. 8, p. 1-12 12 p., 675122.

  Research output › peer-review

  Open Access

• Selective extraction of trivalent actinides using CyMe4BTPhen in the ionic liquid Aliquat-336 nitrate

  Zsabka, P., Van Hecke, K., Adriaensen, L., Wilden, A., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 3 Feb 2021, In: RSC Advances. 11, p. 6014-6021 8 p.

  Research output › peer-review

  Open Access

• Two-step alkaline thorium dioxide precipitation A low waste method for highly sinterable ThO 2

  Wangle, T., Peeters, N., Cautaerts, N., Delloye, T., Cardinaels, T., Vleugels, J. & Verwerft, M., 2 Apr 2021, In: Journal of Nuclear Materials. 552, p. 1-10 10 p., 152984.

  Research output › peer-review

  Open Access
• 2020

  Determination of the lanthanides, uranium and plutonium by means of on-line high-pressure ion chromatography coupled with sector field inductively coupled plasma-mass spectrometry to characterize nuclear samples

  Wanna, N., Van Hoecke, K., Dobney, A., Vasile, M., Cardinaels, T. & Vanhaecke, F., 26 Apr 2020, In: Journal of Chromatography A. 1617, 9 p., 460839.

  Research output › peer-review

  Open Access

• Fabrication of Nd- and Ce-doped uranium dioxide microspheres via internal gelation

  Schreinemachers, C., Leinders, G., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 28 Apr 2020, In: Journal of Nuclear Materials. 535, p. 1-10 10 p., 152128.

  Research output › peer-review

  Open Access

• Gamma Radiolysis of TODGA and CyMe4BTPhen in the Ionic Liquid Tri-n-Octylmethylammonium Nitrate

  Zsabka, P., Van Hecke, K., Wilden, A., Modolo, G., Hupert, M., Jespers, V., Voorspoels, S., Verwerft, M., Binnemans, K. & Cardinaels, T., 20 Jan 2020, (E-pub ahead of print) In: Solvent extraction and ion exchange. 38, 2, p. 212-235 24 p.

  Research output › peer-review

  Open Access

• In Vivo Pharmacokinetics, Biodistribution and Toxicity of Antibody-Conjugated Gold Nanoparticles in Healthy Mice

  Daems, N., Verlinden, B., Van Hoecke, K., Cardinaels, T., Baatout, S., Michiels, C., Lucas, S. & Aerts, A., Jun 2020, In: Journal of Biomedical Nanotechnology. 16, 6, p. 985-996 12 p.

  Research output › peer-review

  Open Access

• Morphology dependent sintering path of nanocrystalline ThO2

  Wangle, T., Belis, M., Tyrpekl, V., Pakarinen, J., Cardinaels, T., Delloye, T., Vleugels, J. & Verwerft, M., 1 Mar 2020, In: Journal of Nuclear Materials. 533, p. 1-10 10 p., 152081.

  Research output › peer-review

  Open Access

• Selective Extraction of Americium from Curium and the Lanthanides by the Lipophilic Ligand CyMe4BTPhen Dissolved in Aliquat-336 Nitrate Ionic Liquid

  Zsabka, P., Van Hecke, K., Cardinaels, T., Wilden, A., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 21 Jan 2020, In: Solvent extraction and ion exchange. 38, 2, p. 1-18 18 p.

  Research output › peer-review

  Open Access

• Solvent Extraction Studies for the Separation of Trivalent Actinides from Lanthanides with a Triazole-functionalized 1,10-phenanthroline Extractant: Solvent Extraction and Ion Exchange

  Zsabka, P., Opsomer, T., Van Hecke, K., Dehaen, W., Wilden, A., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 13 Jul 2020, In: Solvent extraction and ion exchange. 38, 7, p. 719-734 16 p.

  Research output › peer-review

  Open Access

• Structural changes of Nd- and Ce-doped ammonium diuranate microspheres during the conversion to U 1 −y Ln y O 2 ±x: C. Schreinemachers

  Schreinemachers, C., Leinders, G., Podor, R., Lautru, J., Clavier, N., Verwerft, M., Binnemans, K. & Cardinaels, T., 15 Dec 2020, In: Journal of Nuclear Materials. 542, p. 1-12 12 p., 152454.

  Research output › peer-review

  Open Access

• Supported ionic liquid phases for the separation of samarium and europium in nitrate media: Towards purification of medical samarium-153

  Van de Voorde, M., Van Hecke, K., Binnemans, K. & Cardinaels, T., Jan 2020, In: Separation and Purification Technology. 232, p. 1-10 10 p., 115939.

  Research output › peer-review

  Open Access

• The conversion of ammonium uranate prepared via sol-gel synthesis into uranium oxides

  Schreinemachers, C., Leinders, G., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., May 2020, In: Nuclear Engineering and Technology. 52, 5, p. 1013-1021 9 p.

  Research output › peer-review

  Open Access

• Therapeutic Efficacy of 213 Bi-labeled sdAbs in a Preclinical Model of Ovarian Cancer

  Dekempeneer, Y., Caveliers, V., Ooms, M., Gysemans, M., Lahoutte, T., Xavier, C., Lecocq, Q., Maes, K., Covens, P., Miller, B. W., Bruchertseifer, F., Morgenstern, A., Cardinaels, T. & D'huyvetter, M., 19 Jul 2020, In: Molecular Pharmaceutics. 17, 9, p. 3553-3566 14 p.

  Research output › peer-review

  Open Access
• 2019

  Atomic transitions and the first ionization potential of promethium determined by laser spectroscopy

  Studer, D., Heinitz, S., Heinke, R., Naubereit, P., Dressler, R., Guerrero, C., Köster, U., Schumann, D. & Wendt, K., 26 Jun 2019, In: Physical Review A. 99javascript:void(0);, p. 1-8 8 p., 062513.

  Research output › peer-review

  Open Access

• Gold nanoparticles affect the antioxidant status in selected normal human cells.

  Daems, N., Van Hoecke, K., Cardinaels, T., Baatout, S., Aerts, A., Michiels, C., Lucas, S., Penninckx, S. & Nelissen, I., 9 Jul 2019, In: International Journal of Nanomedicine. 14, p. 4991–5015 25 p.

  Research output › peer-review

  Open Access

• Labeling of Anti-HER2 Nanobodies with Astatine-211: Optimization and the Effect of Different Coupling Reagents on Their in Vivo Behavior

  Dekempeneer, Y., Bäck, T., Aneheim, E., Jensen, H., Puttemans, J. & Xavier, C., 21 Jun 2019, In: Molecular Pharmaceutics. 16, 8, p. 3524-3533 10 p.

  Research output › peer-review

  Open Access

• Monte Carlo simulations of pre-clinical SPECT systems with (99m)Tc and (188)Re sources: European Journal of Nuclear Medicine and Molecular Imaging, 46, S829-S830.

  Van Hecke, K., Cardinaels, T. & Vandenberghe, S., 10 May 2019, (In preparation) In: European Journal of Nuclear Medicine and Molecular Imaging. 46, p. S829-S830 2 p.

  Research output › peer-review

• Solvent Extraction of Am(III), Cm(III), and Ln(III) Ions from Simulated Highly Active Raffinate Solutions by TODGA Diluted in Aliquat-336 Nitrate Ionic Liquid

  Zsabka, P., Van Hecke, K., Adriaensen, L., Wilden, A., Modolo, G., Verwerft, M., Binnemans, K. & Cardinaels, T., 4 Feb 2019, In: Solvent extraction and ion exchange. 36, 6, p. 519-541 24 p.

  Research output › peer-review

  Open Access

• Stability of europium(II) in aqueous nitrate media

  Van de Voorde, M., Geboes, B., Van Hecke, K., Cardinaels, T., Vander Hoogerstraete, T. & Binnemans, K., 5 Sep 2019, In: Dalton Transactions. 48, 39, p. 14758-14768 11 p.

  Research output › peer-review

  Open Access

• Studies on the Thoria Fuel Recycling Loop Using Triflic Acid: Effects of Powder Characteristics, Solution Acidity, and Radium Behavior

  Tyrpekl, V., Lommelen, R., Wangle, T., Cardinaels, T., Binnemans, K., Verwerft, M. & Vleugels, J., 7 Jan 2019, In: Journal of Sustainable Metallurgy. 5, 1, p. 118-126 11 p.

  Research output › peer-review

  Open Access

• Zirconium isotope found to be a neutron poison

  Heinitz, S. & Koester, U., 18 Feb 2019, In: Nature Physics. 15, 3, p. 208-209 2 p.

  Research output › peer-review

  Open Access
• 2018

  Homogeneous hydrolysis of thorium by thermal decomposition of urea

  Wangle, T., Tyrpekl, V., Delloye, T., Larcher, O., Pakarinen, J., Cardinaels, T., Vleugels, J. & Verwerft, M., 29 Mar 2018, In: Radiochimica Acta. 106, 8, p. 645-653 9 p.

  Research output › peer-review

  Open Access
• 2016

  Irradiation performance of (Th,Pu)O2 fuel under Pressurized Water Reactor conditions

  Boer, B., Lemehov, S., Wéber, M., Parthoens, Y., Gysemans, M., McGinley, J., Somers, J. & Verwerft, M., 1 Apr 2016, In: Journal of Nuclear Materials. 471, p. 97-109 12 p.

  Research output › peer-review

  Open Access