@book{68a46e628f784e638a087176a4c49d35,
title = "Speciation and solubility calculations for waste relevant radionuclides in Essen and seawaters relevant to Boom Clay conditions: Calculations performed with ThermoChimie database 10d_18Oct2021_SIT_O2",
abstract = "Speciation and solubilities of 27 waste relevant radionuclides in Essen water and seawater are calculated using the thermochemical database {\textquoteleft}ThermoChimie, version 10d_SIT{\textquoteright} which is the current reference database assigned by ONDRAF/NIRAS. These calculations are to be used to replace the past calculations done based on the in-house developed database {\textquoteleft}MOLDATA{\textquoteright}. Calculation results revealed that solubilities of alkaline earth metals, Ni, and Ag may increase in Essen water and seawater compared to the present-day BC water due mainly to the decreased pH and dissolved inorganic carbon content. The impact of using different solution activity coefficient correction models, i.e., between Debye-H{\"u}ckel and SIT on speciation and solubilities of considered radionuclides is minor and only observed in seawater.",
keywords = "Boom Clay, Speciation, Solubility, ThermoChimie, MOLDATA, Essen water, Seawater, Salinity",
author = "Lian Wang",
note = "Score=1 - ER-1177",
year = "2022",
month = nov,
day = "24",
language = "English",
series = "SCK CEN Reports",
publisher = "SCK CEN",
number = "ER-1177",
address = "Belgium",
}